Nanorod Surface Plasmon Enhancement of Laser-Induced Ultrafast Demagnetization

dc.contributor.authorXu, Haitian
dc.contributor.authorHajisalem, Ghazal
dc.contributor.authorSteeves, Geoffrey M.
dc.contributor.authorGordon, Reuven
dc.contributor.authorChoi, Byoung C.
dc.date.accessioned2016-04-22T21:45:20Z
dc.date.available2016-04-22T21:45:20Z
dc.date.copyright2015en_US
dc.date.issued2015-10-30
dc.description.abstractUltrafast laser-induced magnetization dynamics in ferromagnetic thin films were measured using a femtosecond Ti:sapphire laser in a pump-probe magneto-optic Kerr effect setup. The effect of plasmon resonance on the transient magnetization was investigated by drop-coating the ferromagnetic films with dimensionally-tuned gold nanorods supporting longitudinal surface plasmon resonance near the central wavelength of the pump laser. With ~4% nanorod areal coverage, we observe a >50% increase in demagnetization signal in nanorod-coated samples at pump fluences on the order of 0.1 mJ/cm2 due to surface plasmon-mediated localized electric-field enhancement, an effect which becomes more significant at higher laser fluences. We were able to qualitatively reproduce the experimental observations using finite-difference time-domain simulations and mean-field theory. This dramatic enhancement of ultrafast laser-induced demagnetization points to possible applications of nanorod-coated thin films in heat-assisted magnetic recording.en_US
dc.description.reviewstatusRevieweden_US
dc.description.scholarlevelFacultyen_US
dc.description.sponsorshipThis work was supported by the NSERC Discovery Grant program and the NSERC Strategic Project Grant: Development and Validation of a Nanophotonics Simulation Toolbox.en_US
dc.identifier.citationXu, H., Hajisalem, G., Steeves, G.M., Gordon, R. & Choi, B.C. (2015). Nanorod surface plasmon enhancement of laser-induced ultrafast demagnetization. Nature: Scientific Reports, 5(15933), 1-6.en_US
dc.identifier.urihttp://dx.doi.org/10.1038/srep15933
dc.identifier.urihttp://hdl.handle.net/1828/7173
dc.language.isoenen_US
dc.publisherNature: Scientific Reportsen_US
dc.rightsAttribution 2.5 Canada*
dc.rights.urihttp://creativecommons.org/licenses/by/2.5/ca/*
dc.subject.departmentDepartment of Electrical and Computer Engineering
dc.subject.departmentDepartment of Physics and Astronomy
dc.titleNanorod Surface Plasmon Enhancement of Laser-Induced Ultrafast Demagnetizationen_US
dc.typeArticleen_US

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