Raman spectroscopy detects metabolic signatures of radiation response and hypoxic fluctuations in non-small cell lung cancer

dc.contributor.authorVan Nest, Samantha J.
dc.contributor.authorNicholson, Leah M.
dc.contributor.authorPavey, Nils
dc.contributor.authorHindi, Mathew N.
dc.contributor.authorBrolo, Alexandre G.
dc.contributor.authorJirasek, Andrew
dc.contributor.authorLum, Julian J.
dc.date.accessioned2020-11-02T20:57:04Z
dc.date.available2020-11-02T20:57:04Z
dc.date.copyright2019en_US
dc.date.issued2019
dc.description.abstractBackground Radiation therapy is a standard form of treating non-small cell lung cancer, however, local recurrence is a major issue with this type of treatment. A better understanding of the metabolic response to radiation therapy may provide insight into improved approaches for local tumour control. Cyclic hypoxia is a well-established determinant that influences radiation response, though its impact on other metabolic pathways that control radiosensitivity remains unclear. Methods We used an established Raman spectroscopic (RS) technique in combination with immunofluorescence staining to measure radiation-induced metabolic responses in human non-small cell lung cancer (NSCLC) tumour xenografts. Tumours were established in NOD.CB17-Prkdcscid/J mice, and were exposed to radiation doses of 15 Gy or left untreated. Tumours were harvested at 2 h, 1, 3 and 10 days post irradiation. Results We report that xenografted NSCLC tumours demonstrate rapid and stable metabolic changes, following exposure to 15 Gy radiation doses, which can be measured by RS and are dictated by the extent of local tissue oxygenation. In particular, fluctuations in tissue glycogen content were observed as early as 2 h and as late as 10 days post irradiation. Metabolically, this signature was correlated to the extent of tumour regression. Immunofluorescence staining for γ–H2AX, pimonidazole and carbonic anhydrase IX (CAIX) correlated with RS-identified metabolic changes in hypoxia and reoxygenation following radiation exposure. Conclusion Our results indicate that RS can identify sequential changes in hypoxia and tumour reoxygenation in NSCLC, that play crucial roles in radiosensitivity.en_US
dc.description.reviewstatusRevieweden_US
dc.description.scholarlevelFacultyen_US
dc.description.sponsorshipThis work was supported by grant funding from CIHR (258926, AGB, AJ, JJL), CFI (32859, AGB, AJ), The BC Cancer Foundation (JJL) and NSERC CGS-D (SJV). The role of the funders was to provide financial support in equipment and operations costs.en_US
dc.identifier.citationVan Nest, S. J., Nicholson, L. M., Pavey, N., Hindi, M. N., Brolo, A. G., Jirasek, A., … Lum, J. L. (2019) Raman spectroscopy detects metabolic signatures of radiation response and hypoxic fluctuations in non-small cell lung cancer. BMC Cancer, 2019. https://doi.org/10.1186/s12885-019-5686-1en_US
dc.identifier.urihttps://doi.org/10.1186/s12885-019-5686-1
dc.identifier.urihttp://hdl.handle.net/1828/12288
dc.language.isoenen_US
dc.publisherBMC Canceren_US
dc.subjectRaman spectroscopy
dc.subjectNon-small cell lung cancer
dc.subjectHypoxia
dc.subjectReoxygenation
dc.subjectIonizing radiation
dc.subjectImmunofluorescence
dc.subject.departmentDepartment of Physics and Astronomy
dc.subject.departmentDepartment of Chemistry
dc.subject.departmentDepartment of Biochemistry and Microbiology
dc.titleRaman spectroscopy detects metabolic signatures of radiation response and hypoxic fluctuations in non-small cell lung canceren_US
dc.typeArticleen_US

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